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Copper(i) as a reducing agent for the synthesis of bimetallic PtCu catalytic nanoparticles

2023-07-20Artigo científico Acesso aberto
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dc.contributor.authorFernández-Lodeiro, Adrián
dc.contributor.authorLodeiro, Javier Fernández
dc.contributor.authorLosada-Garcia, Noelia
dc.contributor.authorNuti, Silvia
dc.contributor.authorCapelo-Martinez, José Luis
dc.contributor.authorPalomo, Jose M.
dc.contributor.authorLodeiro, Carlos
dc.contributor.institutionLAQV@REQUIMTE
dc.contributor.institutionDQ - Departamento de Química
dc.contributor.pblRSC - Royal Society of Chemistry
dc.date.accessioned2023-10-25T22:20:16Z
dc.date.available2023-10-25T22:20:16Z
dc.date.issued2023-07-20
dc.descriptionThis work was supported by the Spanish Government and the Spanish National Research Council (CSIC) (project PIE 201980E081). J. F. L. thanks FCT for the research contract through the Program DL 57/2016–Norma Transitória. This work was carried out in part through the use of the INL user facilities. The authors thank Dr Jamila Djafari for the conceptualization and design of the graphical abstract. We also thank Ramiro Martínez from Novozymes for the gift of enzymes. Publisher Copyright: © 2023 RSC
dc.description.abstractThis work investigates the potential utilization of Cu(i) as a reducing agent for the transformation of the platinum salt K2PtCl4, resulting in the production of stable nanoparticles. The synthesized nanoparticles exhibit a bimetallic composition, incorporating copper within their final structure. This approach offers a convenient and accessible methodology for the production of bimetallic nanostructures. The catalytic properties of these novel nanomaterials have been explored in various applications, including their use as artificial metalloenzymes and in the degradation of dyes. The findings underscore the significant potential of Cu(i)-mediated reduction in the development of functional nanomaterials with diverse catalytic applications.en
dc.description.versionpublishersversion
dc.description.versionpublished
dc.format.extent9
dc.format.extent1730814
dc.identifier.doi10.1039/d3na00158j
dc.identifier.issn2516-0230
dc.identifier.otherPURE: 72637150
dc.identifier.otherPURE UUID: 8f397b24-6f23-4c26-a8ee-b8a5d9537d61
dc.identifier.otherScopus: 85167519693
dc.identifier.otherWOS: 001040549900001
dc.identifier.otherPubMed: 37638153
dc.identifier.otherPubMedCentral: PMC10448313
dc.identifier.otherORCID: /0000-0001-5582-5446/work/201987752
dc.identifier.urihttp://hdl.handle.net/10362/159274
dc.identifier.urlhttps://www.scopus.com/pages/publications/85167519693
dc.language.isoeng
dc.peerreviewedyes
dc.relationFunding Information: info:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50006%2F2020/PT
dc.relationinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50006%2F2020/PT
dc.relationAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
dc.relationNovel synthetic methodologies for metal nanocatalyst based in Gold, Palladium and Platinum and the study of their catalytic performance in key reactions.
dc.relationalterado para: “Engineering design and synthesis of multifunctional nanoparticles based on combinations of soft and metallic materials, and study of their optical, imaging and biological applications” NANO+DRUGS - Engineering Designed Multifunctional Nanocarries based on a combination of Soft@Metallic Nanoparticles with Anticancer+Antibiotic Smart Drug Delivery. Synthesis, Imaging, Antibacterial and Toxicological Assessments.
dc.relationinfo:eu-repo/grantAgreement/FCT/Concurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020/PTDC%2FQUI-COL%2F1517%2F2020/PT
dc.subjectBioengineering
dc.subjectAtomic and Molecular Physics, and Optics
dc.subjectGeneral Chemistry
dc.subjectGeneral Materials Science
dc.subjectGeneral Engineering
dc.titleCopper(i) as a reducing agent for the synthesis of bimetallic PtCu catalytic nanoparticlesen
dc.typejournal article
degois.publication.firstPage4415
degois.publication.issue17
degois.publication.lastPage4423
degois.publication.titleNanoscale Advances
degois.publication.volume5
dspace.entity.typePublication
oaire.awardNumberUIDP/50006/2020
oaire.awardNumberEXPL/QUI-COL/0263/2021
oaire.awardNumberSFRH/BD/144618/2019
oaire.awardNumberPTDC/QUI-COL/1517/2020
oaire.awardTitleAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
oaire.awardTitleNovel synthetic methodologies for metal nanocatalyst based in Gold, Palladium and Platinum and the study of their catalytic performance in key reactions.
oaire.awardTitlealterado para: “Engineering design and synthesis of multifunctional nanoparticles based on combinations of soft and metallic materials, and study of their optical, imaging and biological applications” NANO+DRUGS - Engineering Designed Multifunctional Nanocarries based on a combination of Soft@Metallic Nanoparticles with Anticancer+Antibiotic Smart Drug Delivery. Synthesis, Imaging, Antibacterial and Toxicological Assessments.
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50006%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/3599-PPCDT/EXPL%2FQUI-COL%2F0263%2F2021/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/OE/SFRH%2FBD%2F144618%2F2019/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/Concurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020/PTDC%2FQUI-COL%2F1517%2F2020/PT
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream3599-PPCDT
oaire.fundingStreamOE
oaire.fundingStreamConcurso para Financiamento de Projetos de Investigação Científica e Desenvolvimento Tecnológico em Todos os Domínios Científicos - 2020
project.funder.identifierhttp://doi.org/10.13039/501100001871
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project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
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project.funder.nameFundação para a Ciência e a Tecnologia
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