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Advanced Technologies Conciliating Desulfurization and Denitrogenation to Prepare Clean Fuels

2024-02-09Recensão Acesso aberto
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dc.contributor.authorFaria, Rui G.
dc.contributor.authorSilva, Dinis
dc.contributor.authorMirante, Fátima
dc.contributor.authorGago, Sandra
dc.contributor.authorCunha-Silva, Luís
dc.contributor.authorBalula, Salete S.
dc.contributor.institutionLAQV@REQUIMTE
dc.contributor.institutionDQ - Departamento de Química
dc.contributor.pblMDPI - Multidisciplinary Digital Publishing Institute
dc.date.accessioned2024-09-25T22:26:12Z
dc.date.available2024-09-25T22:26:12Z
dc.date.issued2024-02-09
dc.descriptionFunding Information: This research work received financial support from the European Union (FEDER funds through COMPETE POCI-01-0145-FEDER-031983). Publisher Copyright: © 2024 by the authors.
dc.description.abstractThe removal of sulfur- and nitrogen-containing compounds present in fuels is and will be crucial to accomplish actual strict regulations to avoid environmental and humanity health adversities. The conventional hydrodesulfurization and hydrodenitrogenation processes conducted by refineries are limited due to severe operating conditions, and even more importantly, they are inefficient for simultaneously removing nitrogen- and sulfur-containing compounds in fuels. On the other hand, non-hydrogen technologies are beneficial in terms of mild operating conditions, and during the last two decades, some successful works have shown that these can be highly effective at efficiently removing both sulfur- and nitrogen-containing compounds from liquid fuels. For more than four decades, extensive research (thousands of publications since the 1980s) has been dedicated to developing remote desulfurization technologies without taking into consideration the presence of a complex fuel matrix, or even taking into account the presence of other harmful pollutant elements, such as nitrogen. Even more recently, several effective non-hydrogen denitrogenation processes have been reported without considering the presence of sulfur compounds. This review paper is a reflection on the limited work that has been successfully performed to simultaneously remove sulfur- and nitrogen-containing compounds from fuels. An evaluation of different methodologies (adsorption, extraction, oxidative (photo)catalysis, ultrasound-assisted oxidation) is presented here. Furthermore, this review intends to define new future strategies that will allow the design of more suitable and economical technologies, effectively conciliating desulfurization and denitrogenation processes to produce more sustainable fuels.en
dc.description.versionpublishersversion
dc.description.versionpublished
dc.format.extent24
dc.format.extent2463043
dc.identifier.doi10.3390/catal14020137
dc.identifier.issn2073-4344
dc.identifier.otherPURE: 99725435
dc.identifier.otherPURE UUID: 1abc5416-c45c-4626-bb3a-ab32339b9b62
dc.identifier.otherScopus: 85186412420
dc.identifier.otherWOS: 001172303200001
dc.identifier.urihttp://hdl.handle.net/10362/172398
dc.identifier.urlhttps://www.scopus.com/pages/publications/85186412420
dc.language.isoeng
dc.peerreviewedyes
dc.relationinfo:eu-repo/grantAgreement/FCT/CEEC IND 2018/CEECIND%2F00793%2F2018%2FCP1545%2FCT0008/PT
dc.relationNot Available
dc.relationNot Available
dc.relationDesigning an alternative technology capable to conciliate efficient desulfurization and denitrogenation processes
dc.relationDesigning a New Route to Promote Desulfurization of Maritime fuels: From Bulk catalysts to Membranes
dc.relationAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
dc.relationinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50006%2F2020/PT
dc.relationinfo:eu-repo/grantAgreement/FCT/Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017%2F2018) - Financiamento Programático/UIDP%2F50006%2F2020/PT
dc.subjectacid rains
dc.subjectadsorption
dc.subjectcatalyst
dc.subjectdenitrogenation
dc.subjectdesulfurization
dc.subjectextraction
dc.subjectfuel
dc.subjectfuels
dc.subjectoxidation
dc.subjectCatalysis
dc.subjectGeneral Environmental Science
dc.subjectPhysical and Theoretical Chemistry
dc.subjectSDG 3 - Good Health and Well-being
dc.subjectSDG 7 - Affordable and Clean Energy
dc.subjectSDG 17 - Partnerships for the Goals
dc.titleAdvanced Technologies Conciliating Desulfurization and Denitrogenation to Prepare Clean Fuelsen
dc.typereview
degois.publication.issue2
degois.publication.titleCatalysts
degois.publication.volume14
dspace.entity.typePublication
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oaire.awardTitleDesigning an alternative technology capable to conciliate efficient desulfurization and denitrogenation processes
oaire.awardTitleDesigning a New Route to Promote Desulfurization of Maritime fuels: From Bulk catalysts to Membranes
oaire.awardTitleAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/CEEC IND 2018/CEECIND%2F00793%2F2018%2FCP1545%2FCT0008/PT
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oaire.awardURIinfo:eu-repo/grantAgreement/FCT/Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017%2F2018) - Financiamento Programático/UIDP%2F50006%2F2020/PT
oaire.fundingStreamCEEC IND 2018
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oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStreamConcurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017/2018) - Financiamento Programático
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