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Alkali-Doped Nanopaper Membranes Applied as a Gate Dielectric in FETs and Logic Gates with an Enhanced Dynamic Response

2023-02-15Artigo científico Acesso aberto
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dc.contributor.authorGaspar, Diana
dc.contributor.authorMartins, Jorge
dc.contributor.authorCarvalho, José Tiago
dc.contributor.authorGrey, Paul
dc.contributor.authorSimões, Rogério
dc.contributor.authorFortunato, Elvira
dc.contributor.authorMartins, Rodrigo
dc.contributor.authorPereira, Luís
dc.contributor.institutionUNINOVA-Instituto de Desenvolvimento de Novas Tecnologias
dc.contributor.institutionCENIMAT-i3N - Centro de Investigação de Materiais (Lab. Associado I3N)
dc.contributor.institutionDCM - Departamento de Ciência dos Materiais
dc.contributor.pblACS - American Chemical Society
dc.date.accessioned2023-07-06T22:16:34Z
dc.date.available2023-07-06T22:16:34Z
dc.date.issued2023-02-15
dc.descriptionFunding Information: The manuscript was written mainly by D.G. with the contributions of all authors. The conceptualization of the work was made by D.G. and L.P. The majority of the experimental work, fabrication, and characterization of the nanopaper was conducted by D.G. with support from P.G. and J.T.C. on the functionalization and electrochemical characterization. The electrical characterization and endurance tests were supported by J.M.. R.S., E.F., R.M., and L.P. were involved in the writing─review and editing of the manuscript. The funding acquisition was ensured by D.G., L.P., E.F., and R.M. This work was supported by LISBOA-05-3559-FSE-000007 and CENTRO-04-3559-FSE-000094 operations, cofunded by the Lisboa2020, Centro 2020 Programme, Portugal 2020, European Union, through the European Social Fund as well as by Fundacao para a Ciencia e Tecnologia (FCT) and Agencia Nacional de Inovacao (ANI). This work was also supported by the FEDER funds through the COMPETE 2020 Program and the National Funds through the FCT-Portuguese Foundation for Science and Technology under Project No. POCI-01- 0145-FEDER-007688, Reference UIDB/50025/2020-2023.The authors would like to acknowledge the European Commission under Project NewFun (ERC-StG-2014). Publisher Copyright: © 2023 The Authors. Published by American Chemical Society.
dc.description.abstractThe market for flexible, hybrid, and printed electronic systems, which can appear in everything from sensors and wearables to displays and lighting, is still uncertain. What is clear is that these systems are appearing every day, enabling devices and systems that can, in the near future, be crumpled up and tucked in our pockets. Within this context, cellulose-based modified nanopapers were developed to serve both as a physical support and a gate dielectric layer in field-effect transistors (FETs) that are fully recyclable. It was found that the impregnation of those nanopapers with sodium (Na+) ions allows for low operating voltage FETs (<3 V), with mobility above 10 cm2 V-1 s-1, current modulation surpassing 105, and an improved dynamic response. Thus, it was possible to implement those transistors into simple circuits such as inverters, reaching a clear discrimination between logic states. Besides the overall improvement in electrical performance, these devices have shown to be an interesting alternative for reliable, sustainable, and flexible electronics, maintaining proper operation even under stress conditions.en
dc.description.versionpublishersversion
dc.description.versionpublished
dc.format.extent8
dc.format.extent6769110
dc.identifier.doi10.1021/acsami.2c20486
dc.identifier.issn1944-8244
dc.identifier.otherPURE: 65371213
dc.identifier.otherPURE UUID: 6529e388-ce70-439d-989f-fb868053b78e
dc.identifier.otherScopus: 85147558764
dc.identifier.otherWOS: 000928781100001
dc.identifier.otherPubMed: 36734958
dc.identifier.otherPubMedCentral: PMC9940104
dc.identifier.otherORCID: /0000-0002-4202-7047/work/151403297
dc.identifier.otherORCID: /0000-0002-7518-0275/work/151408835
dc.identifier.urihttp://hdl.handle.net/10362/154932
dc.identifier.urlhttps://www.scopus.com/pages/publications/85147558764
dc.language.isoeng
dc.peerreviewedyes
dc.relationinfo:eu-repo/grantAgreement/FCT/3599-PPCDT/PTDC%2FNAN-MAT%2F32558%2F2017/PT
dc.relationinfo:eu-repo/grantAgreement/FCT/3599-PPCDT/PTDC%2FCTM-CTM%2F4653%2F2021/PT
dc.relationinfo:eu-repo/grantAgreement/FCT/OE/SFRH%2FBD%2F139225%2F2018/PT
dc.relationSustainable functionalized fiber-based structures for application in electronic and electrochemical systems
dc.relationNew era of printed paper electronics based on advanced functional cellulose
dc.relationSYmbiosis for eNERGY harversting concepts for smart platforms on foils
dc.relationEmerging Printed Electronics Research Infrastructure (EMERGE)
dc.relationinfo:eu-repo/grantAgreement/EC/H2020/101008701/EU
dc.subjectcellulose-based FETs
dc.subjectcellulose-based logic gates
dc.subjectionic doping
dc.subjectnanocellulose
dc.subjectpaper electronics
dc.subjectGeneral Materials Science
dc.titleAlkali-Doped Nanopaper Membranes Applied as a Gate Dielectric in FETs and Logic Gates with an Enhanced Dynamic Responseen
dc.typejournal article
degois.publication.firstPage8319
degois.publication.issue6
degois.publication.lastPage8326
degois.publication.titleACS Applied Materials and Interfaces
degois.publication.volume15
dspace.entity.typePublication
oaire.awardNumberPTDC/NAN-MAT/32558/2017
oaire.awardNumberPTDC/CTM-CTM/4653/2021
oaire.awardNumberSFRH/BD/139225/2018
oaire.awardNumber640598
oaire.awardNumber952169
oaire.awardNumber101008701
oaire.awardTitleSustainable functionalized fiber-based structures for application in electronic and electrochemical systems
oaire.awardTitleNew era of printed paper electronics based on advanced functional cellulose
oaire.awardTitleSYmbiosis for eNERGY harversting concepts for smart platforms on foils
oaire.awardTitleEmerging Printed Electronics Research Infrastructure (EMERGE)
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/3599-PPCDT/PTDC%2FNAN-MAT%2F32558%2F2017/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/3599-PPCDT/PTDC%2FCTM-CTM%2F4653%2F2021/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT//SFRH%2FBD%2F139225%2F2018/PT
oaire.awardURIinfo:eu-repo/grantAgreement/EC/H2020/640598/EU
oaire.awardURIinfo:eu-repo/grantAgreement/EC/H2020/952169/EU
oaire.awardURIinfo:eu-repo/grantAgreement/EC/H2020/101008701/EU
oaire.fundingStream3599-PPCDT
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oaire.fundingStreamH2020
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project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameEuropean Commission
project.funder.nameEuropean Commission
project.funder.nameEuropean Commission
rcaap.rightsopenAccess
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